The sets of core samples were distributed to over 120 laboratories that had returned an original questionnaire seeking expressions of interest in participation. A reporting format for the results was also agreed and distributed to the laboratories at the same time. This is shown in Table 2.1. Laboratories were originally given 1 yr (i.e., to August 2000) to complete the analyses and return the results, but this was later extended to December 2000. In this section, we briefly describe the laboratory characteristics and the overall response rate of the participating laboratories.

Age offsets of accelerator mass spectrometry (AMS) assays on food residue taken from pottery vessels are well-documented in Europe and Asia in cultural contexts were freshwater aquatic products are attested, but are less well studied in North America. The present study examines a series of residue dates from the late prehistoric Central Plains of North America, comparing them with context dates run on annual plant remains. At least 13 of 23 assays are either incongruent with ages on annual plant remains, inconsistent among themselves within a site, or not credible for their cultural context. The conclusion is that food residue from ceramics does not produce consistently accurate dates. Some possible factors that may serve to introduce old carbon to residue samples are discussed. It also is noted that one's conclusions about the reliability of residue may be conditioned by the precision of the age determinations and by the goals of a specific chronology-building effort.

A new facility for radiocarbon dating by accelerator mass spectrometry (AMS) was established in early 2015 at the Inter-University Accelerator Centre in New Delhi, India. The facility uses a 500 kV National Electrostatic Corporation (NEC) Pelletron accelerator for AMS measurements on graphite produced using the automated graphitization equipment (AGE) interfaced with an elemental analyzer and the carbonate handling system (CHS). A precision of better than 1‰ in the ratio of 14C/12C for the modern carbon sample and the background level of 1 × 10–15 from dead carbon sample has been achieved. This is the first dedicated accelerator of India only for AMS activities. This AMS system has the capabilities to perform 10Be and 26Al measurements as well.

Radiocarbon (14C) is a key radionuclide in the assessment of the safety of underground geological disposal facilities for radioactive wastes, and the understanding of the 14C behavior in stainless steel may lead to a re-evaluation of the near-surface repository for the disposal of wastes containing this radionuclide in high concentrations. To achieve this objective, leaching experiments were planned for two different scenarios. The first is where the leaching solution, NaOH solution of pH ca. 12 in aerobic conditions, simulates the expected conditions in a cement-based near-surface repository over long time periods. The other one uses an acid solution of 1M H3PO4, which has been proved as a high efficiency chemical removal agent of 14C in graphite. The development of both analytical methods and protocols to measure the release of 14C from the activated steel samples and the speciation in the aqueous and gaseous phase has been undertaken as part of the EC CAST (CArbon-14 Source Term) project. Analytical methods, suitable for identifying and quantifying low molecular weight organic molecules, comprise ion chromatography (IC) and gas chromatography coupled to mass spectrometry (GC-MS); they are described for aqueous and gaseous samples, respectively. In this paper the preparation of leaching experiments to measure the release of 14C and the results obtained are described.

Radiocarbon analysis of freshwater dissolved organic carbon (DOC) involves substantial sample pretreatment, including an initial rotary evaporation stage necessary to concentrate large volumes of freshwater sample. This may lead to a health risk from the exposure to pathogens, and there is the additional concern that the warm conditions during the rotary evaporation stage may provide ideal growing conditions for some pathogens. To remove any pathogen risk in water samples, boiling or autoclaving can be undertaken. However, to date, no studies have been undertaken to investigate whether boiling will alter the 14C signature of dissolved organic carbon. Here, we analyze the effect of sterilization on 9 contrasting river water samples. Comparing filtered, filtered and boiled, and filtered and sterilized dissolved organic matter, we observe that both boiling and autoclaving increases the uncertainty associated with the 14C and 13C of DOC, that the 14C and 13C changes are not unidirectional, and that they are not related to original DOC composition. Neither sterilization method is recommended unless essential, in which instance we recommend a 3σ uncertainty on 14C and that the 13C is not considered representative of the original sample.

The measurements reported in this date list form the chronometric framework for obsidian hydration and trade studies in California (Ericson, 1975; 1977; 1978; 1981; Ericson et al, 1975; Singer and Ericson, 1977). All samples were analyzed as CO2 gas at close to 1 atm in a 7.5L proportional counter with three energy channels. Radiocarbon ages are based by convention on the 5568 ± 30 yr half-life. The biospheric standard is 95% the count rate of NBS oxalic acid for radiocarbon laboratories. Background is based on CO2 obtained from marble. Counter operation is checked against a historically dated wood sample from the funerary boat of Sesostris III, 1872 +4−8 BC (Hayes, 1962). All samples were subjected to accepted NaOH, HCl or other special chemical treatments to exclude contamination. No tree-ring calibration was applied to any of the samples listed.

The chronologic record of late Quaternary biota from central Alberta has broad implications for understanding the archaeological, geological, paleontological, and paleoenvironmental record of western North America. Radiocarbon dates on remains of Pleistocene megafauna were previously used as proxies for the advance and retreat of ice sheets across Alberta (e.g. Young et al. 1994; Dyke 2005), and are important for understanding landscape changes that likely influenced the timing of human dispersal into North America (Burns 1996). 14C records of Holocene age continue to refine our understanding of landscape change leading up to modern environmental conditions (Beaudoin 2003). Here, we report 15 14C dates from new and previously recorded sites in central Alberta, and one from just across the border within Saskatchewan (Figure 1).

California's Northern Channel Islands have long been an epicenter of specialized fishing economies dating from 13,000 yr ago to the mid-19th century. With thousands of well-preserved shell middens, some dominated by single shellfish species and little to no material culture, it can be difficult to distinguish between specialized prehistoric and historical deposits at some site types. Beginning at least in the Early Holocene and continuing into the Historic period, California mussels, turban snails, and abalone were targeted for specialized collection and processing by Native Americans and later Chinese and Euro-American fishers. Here, we demonstrate how selective accelerator mass spectrometry (AMS) radiocarbon dating of specialized abalone processing camps can help distinguish between prehistoric and historical sites. While unconventional, our case study demonstrates the utility of 14C dating at sites less than 300 yr old.

The complex geographical scenario of Mexico allowed the cultural diversification and development of multiple cultures such as Tolteca, Teotihuacan, Mexica, and Maya, among others. Despite this rich cultural heritage, radiometric dating of Mexican cultural samples with radiocarbon (14C) began only in the 1980s and with accelerator mass spectrometry (AMS) in 2013. Analysis of 14C with AMS is the most widely used technique to date archaeological objects and cultural heritage. Since 2013, the Accelerator Mass Spectrometry Laboratory (LEMA) facility of the Institute of Physics at UNAM (IF-UNAM) has supported archaeological research in Mexico, but also investigation in other areas such as geology, physics, chemistry, and environmental sciences through the analysis of 14C, 10Be, 26Al, 129I, and Pu. The absolute dating with 14C continues to be the core of LEMA’s work, where different geographical scenarios of the country and climatic conditions present very diverse analytical challenges. This work presents a basic description of the AMS system of the LEMA laboratory and describes some applications that are currently being developed.

While assessing the environmental impact of nuclear power plants, researchers have focused their attention on radiocarbon (14C) owing to its high mobility in the environment and important radiological impact on human beings. The 10 MW high-temperature gas-cooled reactor (HTR-10) is the first pebble-bed gas-cooled test reactor in China that adopted helium as primary coolant and graphite spheres containing tristructural-isotropic (TRISO) coated particles as fuel elements. A series of experiments on the 14C source terms in HTR-10 was conducted: (1) measurement of the specific activity and distribution of typical nuclides in the irradiated graphite spheres from the core, (2) measurement of the activity concentration of 14C in the primary coolant, and (3) measurement of the amount of 14C discharged in the effluent from the stack. All experimental data on 14C available for HTR-10 were summarized and analyzed using theoretical calculations. A sensitivity study on the total porosity, open porosity, and percentage of closed pores that became open after irradiating the matrix graphite was performed to illustrate their effects on the activity concentration of 14C in the primary coolant and activity amount of 14C in various deduction routes.

Hikobe House is an important cultural property located in Gunma prefecture. It is one of the oldest manor houses in the Kanto region of Japan. The age of the Hikobe House has up to now been uncertain. There are no architectural records or memorandum tags that indicate when the Hikobe House was built. The living room of the Hikobe House has a style of the latter half of the 17th century, while the guest rooms exhibit a style more typical of the 16th century. So, architectural historians did not agree when the house was built. The wooden materials of the Hikobe House (zelkova, cherry tree, and Japanese red pine) are species that are not well suited to dendrochronology. Thus we investigated the materials of the Hikobe House using the radiocarbon (14C) dating method. Using both the 14C wiggle-match dating method on short tree-ring sequences and observations of remodeling traces of the materials, we were able to establish a credible age of Hikobe House as dating from the late 17th century.

This list contains the results of measurements of 172 radiocarbon samples made between January 1983 and December 1985. An additional 152 samples were measured, but these were submitted without detailed information, such as sample location and sampling depth; therefore, they were excluded from the list.

The radiocarbon revolution may be seen in retrospect as the most decisive development in the archaeology of the 20th century. It is a pleasure, therefore, to have the opportunity of congratulating Radiocarbon on its jubilee celebration, and on the significant role that it has played in establishing a level of excellence in publication, against which the advances in that revolution could be measured. I well remember, as an undergraduate in Cambridge starting to read archaeology in 1960, how each new issue of Radiocarbon would be scrutinized for new dates bearing upon European prehistory. Glyn Daniel, then editor of Antiquity, would often begin a lecture with the announcement of some improbably early date for a Neolithic monument in Brittany or in Britain. It was clear that archaeology was being transformed, but not yet evident what the nature of the transformation would be.

Nowadays, most radiocarbon (14C) laboratories can reliably avoid and remove any possible sample contamination during the pretreatment of organic samples (e.g., bones, charcoal, or trees) thanks to a series of methods commonly used by the radiocarbon community. However, what about the final step, the storage of graphite? Rarely do the laboratories produce their graphite and ship it as pressed targets to accelerator mass spectrometry (AMS) facilities for measurement. Pressed graphite in aluminum targets are vulnerable to contamination, and during shipment or storage, exogenous carbon can be introduced again. Here we report a test on various archaeological sample materials from different environments and different periods (from the past three millennia to the Middle Paleolithic period). We transformed them into graphite, pressed the graphite into targets and sent them to two different AMS laboratories to be dated. We observe that packing details of the targets, extended shipment and storage time may lead to contamination which can be avoided by appropriate packaging in tight metal cans and sealed in vacuum bags. Close cooperation and coordination between our chemistry laboratory and the AMS facilities, high standards in contamination removal, and efficient measurement planning enabled us to obtain reliable 14C ages within a short time.

The dates in this list follow, in approximately chronologic order, those reported in Harwell III (R, 1979, v 21, p 358–383). It is confined to archaeologic samples from the United Kingdom only, most of which originate from “rescue” type operations supported by the Historic Buildings and Monuments Commission for England, (formerly a section of the Dept. of the Environment) and submitted through the Ancient Monuments Laboratory, London.

The radiocarbon dating laboratory of Queens College, CUNY, was established with the joint support of the Research Foundation of the City University of New York and the departments of Anthropology, Biology, Chemistry, and Earth and Environmental Sciences of Queens College. The laboratory has been operational since June, 1975 and is located in the basement of a two-story concrete and brick building.

This radiocarbon laboratory began operation in 1980 using the benzene scintillation method. The benzene synthesizer is essentially identical with that of Ikeda (1976). A liquid scintillation counter is Aloca LSC-LB1. Samples dated are wood, charcoal, shell, and coral.

Pretreatment of wood and charcoal is a standard acid-alkali procedure, using 2% HCl and 2% NaOH at elevated temperatures. Charcoal is further heated in concentrated HNO3 for one hour, diluted in water, stands one night, and is washed and dried. Pretreated wood and charcoal are carbonized before combustion. The combustion products are passed over CuO, and are collected in an ammonium hydroxide bubbler system, and precipitated with calcium chloride.