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Plasmonic metal–semiconductor heterostructures for hot-electron-driven photochemistry

Published online by Cambridge University Press:  10 January 2020

Jiawei Huang ,
Wenxiao Guo ,
Yue Hu  and
Wei David Wei
Jiawei Huang
Affiliation:
Department of Chemistry, University of Florida, USA; [email protected]
Wenxiao Guo
Affiliation:
Department of Chemistry, University of Florida, USA; [email protected]
Yue Hu
Affiliation:
Department of Chemistry, University of Florida, USA; [email protected]
Wei David Wei
Affiliation:
Department of Chemistry, University of Florida, USA; [email protected]
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Abstract

Plasmonic nanostructures possess broadly tunable optical properties with catalytically active surfaces. They offer new opportunities for achieving efficient solar-to-chemical energy conversion. Plasmonic metal–semiconductor heterostructures have attracted heightened interest due to their capability of generating energetic hot electrons that can be collected to facilitate chemical reactions. In this article, we present a detailed survey of recent examples of plasmonic metal–semiconductor heterostructures for hot-electron-driven photochemistry, including plasmonic metal–oxide, plasmonic metal–two-dimensional materials, and plasmonic metal–metal–organic frameworks. We conclude with a discussion on the remaining challenges in the field and an outlook regarding future opportunities for designing high-performance plasmonic metal–semiconductor heterostructures for photochemistry.

Type
Materials for Hot-Carrier Chemistry
Information
MRS Bulletin , Volume 45 , Issue 1: Materials for Hot-Carrier Chemistry , January 2020 , pp. 37 - 42
Copyright
Copyright © Materials Research Society 2020

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