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  3. Nonlinear Optical Polarization Analysis in Chemistry and Biology
  • Cited by 19
Publisher:
Cambridge University Press
Online publication date:
May 2017
Print publication year:
2017
Online ISBN:
9781139019026
DOI:
https://doi.org/10.1017/9781139019026
Subjects:
Optics, Optoelectronics and Photonics, Physics and Astronomy, Engineering, Physical Chemistry, Atomic Physics, Molecular Physics and Chemical Physics, Materials Science
Product:
Materials Research Society
Series:
Cambridge Molecular Science
Information

Book description

This rigorous yet accessible guide presents a molecular-based description of nonlinear optical polarization analysis of chemical and biological assemblies. It includes discussion of the most common nonlinear optical microscopy and interfacial measurements used for quantitative analysis, specifically second harmonic generation (SHG), two-photon excited fluorescence (2PEF), vibrational sum frequency generation (SFG), and coherent anti-Stokes Raman spectroscopy/stimulated Raman spectroscopy (CARS/SRS). A linear algebra mathematical framework is developed, allowing step-wise systematic connections to be made between the observable measurements and the molecular response. Effects considered include local field corrections, the molecular orientation distribution, rotations between the molecular frame, the local frame and the laboratory frame, and simplifications from molecular and macromolecular symmetry. Specific examples are provided throughout the book, working from the common and relatively simple case studies through to the most general scenarios.

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