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Evaluation of radionuclides in groundwater around proposeduranium mining sites in Bagjata and Banduhurang, Jharkhand (India)

Published online by Cambridge University Press:  09 March 2011

S. Giri
Affiliation:
Dept. of Environmental Science and Engineering, Indian School of Mines, Dhanbad-826004, India
G. Singh
Affiliation:
Dept. of Environmental Science and Engineering, Indian School of Mines, Dhanbad-826004, India
V. N. Jha
Affiliation:
Environmental Assessment Division, Bhabha Atomic Research Centre, Mumbai-400085, India
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Abstract

Radionuclides find their way into the water resources at sites in the vicinity of nuclearfacilities involved in mining, milling, ore separation, purification, etc. The presentedstudy delineates the distribution of radionuclides {Ra and U(nat)} in groundwatersexisting in the vicinity of two proposed uranium mine sites and evaluates their ingestiondose through the intake of drinking water. The study reveals that the U(nat) concentrationin groundwater varied from <0.5 to 11.2μg.l-1 in the Bagjata mining area and from<0.5 to 27.5 μg.l-1 in theBanduhurang mining area, while 226Ra was found in the range of <3.5 to 206 mBq.l-1 and<3.5 to 82 mBq.l-1, respectively, for both areas.Seasonal variation and distribution of radionuclides in the study area did not show anydefinite pattern. A strong positive correlation of U(nat) in groundwater with pH andnegative correlation of 226Ra with pH is shown in the study. The ingestion doseto the public through intake of drinking water is estimated as 9.43μSv.y-1 for Bagjata and 6.28μSv.y-1 for Banduhurang, which is much lower than thereference limit (100 μSv.y-1) given by the WHO.

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Article
Copyright
© EDP Sciences, 2011

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References

Références

Almeida, R.M.R., Lauria, D.C., Ferreira, A.C., Sracek, O. (2004) Groundwater radon, radium and uranium concentrations in Região dos Lagos, Rio de Janeiro State, Brazil, J. Environ. Radioact. 73, 323-334. Google Scholar
Bansal, V., Tyagi, R.K., Prasad, R. (1988) Determination of uranium concentration in drinking water samples by fission track method, J. Radioanal. Nucl. Chem. 125, 439-443. Google Scholar
Benes P. (1990) Radium in (Continental) Surface Water, The Environmental Behavior of Radium. Technical Reports Series No. 310, International Atomic Energy Agency, Vienna, pp. 373-418.
Bhola K.L., Dar K.K., Ramarao Y.N., Suri Sastry C., Mehta N.R. (1964) A review of Uranium and Thorium deposits in India. In: Proceedings of 3rd International Conference of the peaceful uses of Atomic Energy. Multilingual Edition United Nations, Volume 12, pp. 750-756.
Bou-Rabee, F. (1995) Estimating the concentration of uranium in some environmental samples in Kuwait after the 1991 gulf war, Appl. Radiat. Isotopes 46, 217-220. Google Scholar
Brown, A., Steenfelt, A., Kunzennorf, H. (1983) Uranium districts defined by reconnaissance geochemistry in south Greenland, J. Geochem. Explor. 19, 127-145. Google Scholar
Brunke, M., Gonser, T. (1997) The ecological significance of exchange processes between rivers and ground-water, Freshw. Biol. 37, 1-33. Google Scholar
Burcik, I., Mikulaj, V. (1991) Separation of Thorium, Uranium and Plutonium by Neutral and Basic Organic Extractants, J. Radioanal. Nucl. Chem. 5, 247-255. Google Scholar
Butler A.H., Kahn B. (1995) Radon-222, Radium-226 and Uranium in Georgia Piedmont well water. In: Proceedings of the 1995 Georgia Water Resources Conference, April 11-12, 1995, Athens.
Correia J.A., Weise S.B., Callahan R.J., Strauss H.W. (1987) The Kinetics of Ingested 222Rn in Humans Determined from Measurements with 133X. Cooperative Agreement # CR 8109427, U.S. EPA, Health Affects Research Laboratories, Cincinnati, OH.
Cothern, C.R., Lappenbusch, W.L. (1983) Occurrence of uranium in drinking water in the US, Health Phys. 45, 89-99. Google Scholar
Dang H.S., Jaiswal D.D., Parameswaran M., Krishnamony S. (1994) Physical Anatomical, Physiological and Metabolic Data for Reference Man-A Proposal. BARC/1994/E/043.
DePaul V.T., Szabo Z. (2007) Occurrence of Radium-224, Radium-226 and Radium-228 in Water from the Vincentown and Wenonah-Mount Laurel Aquifers, the Englishtown Aquifer System, and the Hornerstown and Red Bank Sands, Southwestern and South-Central New Jersey. Scientific Investigations Report 2007-5064, Prepared in cooperation with the New Jersey Department of Environmental Protection.
Fentiman A.W., Smith M., Veley R.J. (2004) How do radioactive materials move through the environment to people? Ohio State University Extension. www.ag.ohio-state.edu/rer /rerhtml/rer 25.html
Firestone B.R., Shirley M.C., Baglin Y.S., Frank Chu, Zipkin J. (1996) The 8th Edition of the Table of Isotopes. CD-ROM, JohnWiley & Sons, Inc.
Gascoyne, M. (1989) High Levels of Uranium and Radium in Groundwater at Canada’s Underground, Appl. Geochem. 4, 557-591. Google Scholar
Gilkeson, R.H., Cartwright, K., Cowart, J.B., Holtzman, R.B. (1983) Hydrogeologic and geochemical studies of selected natural radioisotopes and barium in groundwater in Illinois, Illinois Department of Energy and Natural Resources report 6, 93. Google Scholar
Goode, D.J., Wilder, R.J. (2006) Ground-Water Contamination near a Uranium Tailings Disposal Site in Colorado, J. Ground Water 25, 545-554. Google Scholar
Hoffmann, W., Kranefeld, A., Schmitz-Feuerhake, I. (1993) Radium-226 contaminated Drinking water: Hypothesis on an Exposure Pathway in a Population with Elevated Childhood Leukemia, Environ. Health Persp. Suppl. 101, 113-115. Google Scholar
Hsi, C.D., Langmuir, D. (1985) Adsorption of Uranyl onto Ferric Oxyhydroxides: Application of the Surface Complexation Site-Binding Model, Geochim. Cosmochim. Acta 49, 1931-1941. Google Scholar
IAEA (1989) International Atomic Energy Agency. Measurement of radionuclides in food and the environment: A guidebook. IAEA Technical Reports Series, 295. IAEA, Vienna.
ICRP Publication 68 (1994) International Commission on Radiological Protection. Dose Coefficients for Intakes of Radionuclides by Workers, Ann. ICRP 24(4). PubMed
ICRP Publication 69 (1995) International Commission on Radiological Protection. Age–dependent Doses to Members of the Public from Intake of Radionuclides: Part 3 Ingestion Dose Coefficients, Ann. ICRP 25(1). PubMed
ICRP Publication 72 (1996) International Commission on Radiological Protection. Age dependent doses to the members of the public from intake of radionuclides: Part 5, Ann. ICRP 25(2).
Iyengar M.A.R. (1990) The Natural Distribution of Radium, The Environmental Behavior of Radium. Technical Reports Series No. 310, IAEA 1, 9-128.
Kaye G.W.C., Laby T.H. (1993) Tables of physical and chemical constants. Longman Group Ltd, 15th edition, Essex, UK.
Kolthoff I.M., Elving P.J. (1962) Treatise on Analytical Chemistry, part II, Vol. 9.
Kumru, M.N. (1995) Distribution of Radionuclides in sediments and soils along the Buyuk Menderes River, Proc. Pakistan Acad. Sci. 32, 51-56. Google Scholar
Labidi, S., Dochraoui, M., Mahjoubi, H., Lemaitre, N., Ben Salah, R., Mtimet, S. (2002) Natural Radioactive Nuclides in Some Tunisian Thermo-Mineral Springs, J. Environ. Rad. 62, 87-96. Google ScholarPubMed
Lauria, D.C., Almeida, R.M.R., Sracek, O. (2004) Behavior of radium, thorium and uranium in groundwater near the Buena Lagoon in the Coastal Zone of the State of Rio de Janeiro, Brazil, Environmental Geology 47, 11-19. Google Scholar
Lydie, R.M., Nemba, R.M. (2008) Quantitative Determination of 226Ra and 228Ra in Reservoir and Tap Water in Yaounde Area, Cameroon, Global Journal of Environmental Research 2, 110-113. Google Scholar
Mackenzie J.M.W. (1997) Uranium Solvent Extraction Using Tertiary Amines. In: Uranium Ore Yellow Cake Seminar. February 1997 Melbourne, Australia.
Mahesh H.M., Avadhani D.N., Somashekarappa H.M., Karunakara N., Narayana Y., Siddappa K. (2002) Uranium and Radium concentration in ground water in the environment of coastal Karnataka and Kaiga. In: Proceedings National Symposium in Environment-XI, pp. 123-127.
Malcome-Lawes D.J. (1979) Introduction to Radiochemistry. Unwin Brothers Ltd.
Marovic, G., Sencar, J., Franic, Z., Lokobaner, N. (1996) Radium-226 in Thermal and mineral Springs of Croatia and Associated Health Risk, J. Environ. Rad. 33, 309-317. Google Scholar
Nour Khalifa, A. (2004) Natural Radioactivity of Ground and drinking water in some areas of Upper Egypt, Turkish. J. Eng. Env. Sci. 28, 345-354. Google Scholar
Paschoa A.S., Baptista G.B., Montenegro E.C., Miranda A.C., Sigaud G.M. (1979) Radium-226 Concentrations in the Hydrographic Basins near Uranium Mining and Milling in Brazil. In: Proc. of the Mid Year Topical Symposium, Low Level Radioactive Waste Management, Williamsburg, VA, pp. 337-343.
Pulhani, V.A., Dafauti, S., Hegde, A.G. (2007) Leaching of uranium, radium and thorium from vertisol soil by ground water, J. Radioanal. Nucl. Chem. 274, 341-343. Google Scholar
Raghavayya, M., Iyengar, M.A.R., Markose, P.M. (1980) Estimation of Radium-226 by Emanometry, Bull. IARP 3(4). Google Scholar
Rani, A., Singh, S. (2006) Analysis of uranium in drinking water samples using laser induced fluorimetry, Health Phys. 91, 101-107. Google ScholarPubMed
Rout, K.C., Mishra, P.K., Chakravorty, V., Dash, K.C. (1994) Liquid-liquid extraction of uranium(VI) by Cyanex 301/Alamine 308 and their mixtures with TBP/DDSO, J. Radioanal. Nucl. Chem. 181, 3-10. Google Scholar
Salonen, L. (1988) Natural Radionuclides in Groundwater in Finland, Radiat. Prot. Dosim. 24, 163-166. Google Scholar
Santschi, P.H., Hoehn, E., Lueck, A., Farrenkothen, K. (1987) Tritium as a tracer for the movement of surface water and groundwater in the Glatt valley, Switzerland, Environ. Sci. Technol. 21, 909-916. Google Scholar
Schwarzenbach, R.P., Giger, W., Hoehn, E., Schneider, J.K. (1983) Behavior of organic compounds during infiltration of river water to groundwater, Environ. Sci. Technol. 17, 472-479. Google Scholar
Shiraishi, K., Igarashi, Y., Takaku, Y., Masuda, K., Yoshimizu, K., Nishimura, Y., Hongo, S., Yamaguchi, H. (1992) Daily intakes 232Th and 238U in Japanese male, Health Phys. 63, 187-191. Google Scholar
Sidhu, K.S., Breithart, M.S. (1998) Naturally Occurring Radium-226and Radium-228 in Water Supplies of Michigan, Bull. Environ. Contam. Toxicol. 61, 722-729. Google ScholarPubMed
Silva P.S.C., Damatto S.R., Mazzilli B.P. (2008) Sequential Determination of U and Th Decay Series in Santana Cave, Southwest Brazil. In: The Natural Radiation Environment: 8th International Symposium (NRE VIII). AIP Conference Proceedings, 1034, pp. 256-259. CrossRef
Smith B., Powell A.E., Milodowski A.E., Hards V.L., Hutchins M.G., Amro A., Gedeon R., Kilani S., Scrivens S.M., Galt V. (2000) Identification, investigation and remediation of ground water containing elevated levels of uranium-series radionuclides: A case study from the Eastern Mediterranean. In: Proc. of the 3rd Int. Conf. on the geology of the eastern Mediterranean, Nicosia, Cyprus. Geneva: WHO/SDE/PH/01.1.
Sophocleous, M. (2002) Interactions between groundwater and surface water: the state of the science, Hydrogeology Journal 10, 52-67. Google Scholar
Szabo Z., Zapecza O.S. (1991) Geologic and Geochemical Factors Controlling Uranium, Radium-226, and Radon-222 in Ground Water, Newark Basin, New Jersey. In: Field Studies of Radon in Rocks, Soils, and Water, (Gundersen L.C.S., Wanty R.B., eds.) U.S. Geological Survey Bulletin. pp. 243-266.
Tripathi R.M., Sahoo S.K., Jha V.N., Khan A.H., Puranik V.D. (2007) Assessment of Environmental radioactivity at uranium mining, processing and tailings management facility at Jadugoda, India. In: Proc. of Int. Conf. on Environmental Radioactivity during April 23- 28, 2007 at IAEA, Vienna.
Ulbak, K., Klinder, O. (1984) Radium and Radon in Danish Drinking Water, Radiat. Prot. Dosim. 7, 87-89. Google Scholar
UNSCEAR (2000) United Nations Sources and Effects of Ionising Radiation, Report to the General Assembly with Scientific Annexes, United Nations, New York. Vol. 1, pp. 126-127.
US Geological Survey and New Jersey Dept of Env. Protection (2004) Occurrence of Radium-224, Radium-226 and Radium-228 in water of the unconfined Kirkwood-Cohansey Aquifer system, Southern New Jersey. Scientific Investigations.
USEPA (1976) Determination of Radium Removal Efficiencies in Water Treatment Process. Technical Note. ORP/TAD-76-5 Illinois, EPA, Springfield. http://www.epa.gov.
Vesterbacka, P., Turtiainen, T., Heinävaara, S., Arvela, H. (2006) Activity concentrations of 226Ra and 228Ra in drilled well water in Finland, Radiat. Prot. Dosim. 121, 406-412. Google ScholarPubMed
Wanty, R.B., Johnson, S.L., Briggs, P.H. (1991) Radon-222 and its parent radionuclides in groundwater from two study areas in New Jersey and Maryland, U.S.A., Appl. Geochem. 6, 305-318. Google Scholar
Weihai, Z., Takao, I., Xiaotang, Y. (2001) Occurrence of Rn-222, Ra-226, Ra-228 and U in Groundwater in Fujian Province, China, J. Environm. Radioact. 53, 111-120. Google Scholar
Whittemore D.O., McElwee C.D., Tsu M.S. (2000) Arkansas River salinity and contamination of the High Plains aquifer (W.O. Deason, T.K. Gates, D.D. Zimbelman, S.S. Anderson, eds) Challenges facing irrigation and drainage in the new millennium. In: Proc 2000 USCID Intl Conf, Fort Collins, CO. 1, 225-246.
WHO (1978) Radiological Examination of Drinking Water, World Health Organization, Copenhagen.
WHO (1993) Guidelines for drinking water quality. World Health Organization, Geneva.
WHO (2004) Guidelines for Drinking-water Quality: Recommendations by World Health Organization, Edition: 3, Published by World Health Organization.
Wrenn, M.E., Durbin, P.W., Howard, B., Lipsztein, J., Rundo, J., Still, E.T., Willis, D.I. (1985) Metabolism of Ingested U and Ra, Health Phys. 48, 601-633. Google ScholarPubMed