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Diffusion Measurements of Radionuclides In site Specific Sediment/Groundwater-Systems

Published online by Cambridge University Press:  28 February 2011

Hans Meier ,
E. Zimmerhackl ,
G. Zeitler  and
P. Menge
Hans Meier
Affiliation:
Staatliches Forschungsinstitut für Geochemie/Außenstelle des Bayerischen Geologischen Landesamtes, Concordiastraße 28, D-8600 Bamberg, Federal Republic of Germany
E. Zimmerhackl
Affiliation:
Staatliches Forschungsinstitut für Geochemie/Außenstelle des Bayerischen Geologischen Landesamtes, Concordiastraße 28, D-8600 Bamberg, Federal Republic of Germany
G. Zeitler
Affiliation:
Staatliches Forschungsinstitut für Geochemie/Außenstelle des Bayerischen Geologischen Landesamtes, Concordiastraße 28, D-8600 Bamberg, Federal Republic of Germany
P. Menge
Affiliation:
Staatliches Forschungsinstitut für Geochemie/Außenstelle des Bayerischen Geologischen Landesamtes, Concordiastraße 28, D-8600 Bamberg, Federal Republic of Germany
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Abstract

Results of systematic measurements on the diffusion of radionuclides through sandy, marlaceous and clayley sediment rocks from strata overlying the Gorleben salt dome are presented. The tracer nuclides used were U-233, Ra-226, Pb-210, and Ni-63. It is shown that, among other parameters, diffusion coefficients and distribution coefficients could be derived from breakthrough curves. Moreover, it is demonstrated that the diffusion behaviour of nuclides such as Pb and Ni can be enhanced enormously in sediment rocks by complex forming agents (EDTA).

Type
Research Article
Information
MRS Online Proceedings Library (OPL) , Volume 212: Symposium P – Scientific Basis for Nuclear Waste Management XIV , 1990 , 617
Copyright
Copyright © Materials Research Society 1991

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References

REFERENCES

1. Eriksen, T.E. and Jacobsson, A., Report SKBF/KBS 1984–06–28, Stockholm 1984.Google Scholar
2. Lever, D.A. and Bradbury, M.H., Mineral. Mag. 49, 245 (1985).CrossRefGoogle Scholar
3. Torstenfeld, B. and Allard, B., Report KBS TR 86–14, Stockholm 1986.Google Scholar
4. Meier, H., Zimmerhackl, E., Hecker, W., Zeitler, G., Menge, P., Radiochim. Acta 44 /45, 239 (1988).CrossRefGoogle Scholar
5. Warnecke, E., Tittel, G., Brennecke, P., Stier-Friedland, G., Hollmann, A., in IAEA-SM-289/49, 1986, p. 401.Google Scholar
6. Maas, K.E. and Huf, E. (eds.), Proc. U.S./FRG Bilateral Workshop Oct.25, 1982 (Projektstab PSE, HMI Berlin, 1983).Google Scholar
7. Meier, H., Zimmerhackl, E., Zeitler, G., Menge, P., Hecker, W., J. Radioanal. Nucl. Chem., Articles 109, 139 (1987).CrossRefGoogle Scholar
8. Bradbury, M.H., Lever, D., Kinsey, D., in Scientific Basis for Nuclear Waste Management V, edited by Lutze, W. (Elsevier Science Publishers, New York 1982) p. 569.Google Scholar
9. Mills, R. and Lobo, V.M.M., Self-Diffusion in Electrolyte Solutions (Elsevier Science Publishers, New York 1989).Google Scholar
10. Meier, H., Zimmerhackl, E., Zeitler, G., Menge, P., in Proc. U.S./FRG Bilateral Workshop, Oct. 25, 1982, ed. by Maas, K.-E. and Huf, E. (Projektstab PSE, HMI Berlin)(1983) p.37.Google Scholar
11. Meier, H., Zimmerhackl, E., Zeitler, G., Menge, P., Radiochim. Acta 1990 (in press).Google Scholar