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Modeling of Glass Dissolution and Transport With the Code SUGAR

Published online by Cambridge University Press:  10 February 2011

J.S. Small ,
D.P. Trivedi  and
P.K. Abraitisti
J.S. Small
Affiliation:
British Nuclear Fuels plc, Environmental Assessments, R002, Risley, Warrington, U.K.WA3 6AS
D.P. Trivedi
Affiliation:
British Nuclear Fuels plc, Environmental Assessments, R002, Risley, Warrington, U.K.WA3 6AS
P.K. Abraitisti
Affiliation:
Dept of Earth Sciences, The University of Manchester, Manchester, U.K.M13 9PL
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Abstract

SUGAR (Simplified Understading of Glass And environment Reactions) is a one dimensional (lD) reactive transport code which sequentially couples dissolved chemical species transport and sorption with, chemical speciation, mineral precipitation and kinetic controlled glass dissolution. SUGAR also has the capability to model radioactive decay and steel corrosion. This paper describes the computer model and presents results of model testing against experimental data. The capabilities of the model are demonstrated by a preliminary investigation of the geochemical evolution of glass in crystalline rock formations.

Type
Research Article
Information
MRS Online Proceedings Library (OPL) , Volume 506: Symposium – Scientific Basis for Nuclear Waste Management XXI , 1997 , 253
Copyright
Copyright © Materials Research Society 1998

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References

REFERENCES

[1] Grambow, B., Mat. Res. Soc. Symp. Proc. 44, 15–27 (1989).Google Scholar
[2] Aagaard, P. and Helgeson, H. C.. American Journal of Science. 282, 237–285, (1982).Google Scholar
[3] Advocat, T., Crovisier, J.L., Clement, A., Gerard, F., Vernaz, E., Mat. Res. Soc. Symp. Proc. 353, 31–38 (1995)Google Scholar
[4] Yeh, G.T. and Tripathi, V.S., Water Resources Research. 25, 93–108, (1989).Google Scholar
[5] Parkhurst, D.L. Thorstenson, D.C. and Plummer, L.N. PHREEQE - A Computer Program for Geochemical Calculations. U.S. Geological Survey, 1984.Google Scholar
[6] Bourcier, W. L., Peiffer, D. W., Knauss, K. G., McKeegan, K., K., D. and , Smith, Mat. Res. Soc. Syinp. Proc. 176, 209–216, (1990).Google Scholar
[7] Cross, J.E. et al. AERE Rep No. AERE R12324, 1987.Google Scholar
[8] Abraitis, P.K., Vaughan, D.J., Livens, F.R., Monteith, J., Trivedi, D., and Small, J., Dissolution of a complex borosilicate glass at 60°C: The influence of pH and proton adsorption on the congruence of short-term leaching. Mat. Res. Soc. Symp. Proc. (this volume).Google Scholar
[9] Bates, J.K., Ebert, W.L., X.Feng, and Bourcier, W.L., L., W. Journal of Nuclear Materials, 190, 198–227, (1992).Google Scholar