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Magnetic X-Ray Circular Dichroism in Spin-Polarized Photoelectron Diffraction

Published online by Cambridge University Press:  15 February 2011

G. D. Waddill
Affiliation:
Lawrence Livermore National Laboratory, Chemistry and Materials Science Department, P.O. Box 808, L-357, Livermore, CA 94550 ° USA
J. G. Tobin
Affiliation:
Lawrence Livermore National Laboratory, Chemistry and Materials Science Department, P.O. Box 808, L-357, Livermore, CA 94550 ° USA
X. Guo
Affiliation:
University of Wisconsin-Milwaukee, Laboratory for Surface Studies and Department of Physics, Milwaukee, MI 53201 • USA
S. Y. Tong
Affiliation:
University of Wisconsin-Milwaukee, Laboratory for Surface Studies and Department of Physics, Milwaukee, MI 53201 • USA
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Abstract

The first structural determination with spin-polarized, energy-dependent photoelectron diffraction using circularly-polarized x-rays is reported for Fe films on Cu(001). Circularly-polarized x-rays produce spin-polarized photoelectrons from the Fe 2p doublet, and intensity asymmetries in the 2p3/2 level are observed. Fully spin-specific multiple scattering calculations reproduce the experimentally-determined energy and angular dependences. A new analytical procedure which focuses upon intensity variations due to spin-dependent diffraction is introduced. A sensitivity to local geometric and magnetic structure is demonstrated.

Type
Research Article
Copyright
Copyright © Materials Research Society 1995

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