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In situ mapping of chemical segregation using synchrotron x-ray imaging

Published online by Cambridge University Press:  10 November 2020

Shikang Feng ,
Enzo Liotti ,
Matthew D. Wilson ,
Lydia Jowitt  and
Patrick S. Grant
Shikang Feng
Affiliation:
Department of Materials, University of Oxford, UK; [email protected]
Enzo Liotti
Affiliation:
Department of Materials, University of Oxford, UK; [email protected]
Matthew D. Wilson
Affiliation:
Detector Development Group, Rutherford Appleton Laboratory, UK; [email protected]
Lydia Jowitt
Affiliation:
Detector Development Group, Rutherford Appleton Laboratory, UK; [email protected]
Patrick S. Grant
Affiliation:
University of Oxford, UK; [email protected]
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Abstract

Synchrotron x-rays are a powerful tool to probe real-time changes in the microstructure of materials as they respond to an external stimulus, such as phase transformations that take place in response to a change in temperature. X-ray imaging techniques include radiography and tomography, and have been steadily improved over the last decades so that they can now resolve micrometer-scale or even finer structural changes in bulk specimens over time scales of a second or less. Under certain conditions, these imaging approaches can also give spatially resolved chemical information. In this article, we focus on the liquid to solid transformation of metallic alloys and the temporal and spatial resolution of the accompanying segregation of alloying elements. The solidification of alloys provides an excellent case study for x-ray imaging because it is usually accompanied by the progressive, preferential segregation of one or more of the alloying elements to either the solid or the liquid, and gives rise to surprisingly complex chemical segregation patterns. We describe chemical mapping investigations of binary and quasi-binary alloys using radiography and tomography, and recent developments in x-ray fluorescence imaging that offer the prospect of a more general, multielement mapping technique. Future developments for synchrotron-based chemical mapping are also considered.

Type
Processing Metallic Materials Far from Equilibrium
Information
MRS Bulletin , Volume 45 , Issue 11: Processing Metallic Materials Far from Equilibrium , November 2020 , pp. 934 - 942
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Copyright
Copyright © The Author(s), 2020, published on behalf of Materials Research Society by Cambridge University Press

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