Hostname: page-component-cd9895bd7-lnqnp Total loading time: 0 Render date: 2024-12-28T16:16:39.823Z Has data issue: false hasContentIssue false

Mineral dust in urban air: Beijing, China

Published online by Cambridge University Press:  05 July 2018

A. G. Whittaker*
Affiliation:
School of Biosciences, Cardiff University, PO Box 911, Cardiff CF10 3US, UK
T. P. Jones
Affiliation:
School of Biosciences, Cardiff University, PO Box 911, Cardiff CF10 3US, UK
L. Shao
Affiliation:
Department of Fossil Fuel Geological Engineering, Beijing Graduate School, Xueyuan Road, Beijing, P. R. China
Z. Shi
Affiliation:
Department of Fossil Fuel Geological Engineering, Beijing Graduate School, Xueyuan Road, Beijing, P. R. China
K. A. Bérubé
Affiliation:
School of Biosciences, Cardiff University, PO Box 911, Cardiff CF10 3US, UK
R. J. Richards
Affiliation:
School of Biosciences, Cardiff University, PO Box 911, Cardiff CF10 3US, UK

Abstract

The PM10 (airborne particulate matter with aerodynamic diameter <10 mm) in Beijing has a distinct seasonality, with industrial, domestic and natural sources providing a heterogeneous cocktail of airborne particulate matter (PM). Collections were made during late winter, summer and high wind dust storms to determine composition and probable sources of this PM. The concentration of the PM during winter (174 μg m–3) was approximately four times higher than summer (37 μg m–3) with dust storms raising the concentration further (200 μg m–3). During the winter the PM was dominated by combustion products (66% filter area). During the summer combustion products and loess contributed ~35% to the filter area each, but during elevated wind speeds (>10 mph) loess completely dominated the collections (96% filter area). The majority of the PM10 collected was in the respirable (PM2.5) size range (winter 99.7%, summer 96.6%, dust storms 82.3%). The loess in Beijing comprises quartz, feldspar, calcite, chlorite and mica and is in the coarse silt to sand (20–60 mm) size range. The collections are therefore likely to be made up of finer silt and clay, primarily derived from of the erosion of cultivated land. Using a plasmid assay, the Beijing particulate matter was found to have little or no surface free radical activity.

Type
Research Article
Copyright
Copyright © The Mineralogical Society of Great Britain and Ireland 2003

Access options

Get access to the full version of this content by using one of the access options below. (Log in options will check for institutional or personal access. Content may require purchase if you do not have access.)

References

BeruBe, K.A., Jones, T.P., Williamson, B.J., Winters, C., Morgan, A.J. and Richards, R.J. (1999) Physicochemical characterisation of diesel exhaust particles: factors for assessing biological activity. Atmospheric Environment, 33, 15991614.CrossRefGoogle Scholar
Borja-Aburto, V.H., Castillejos, M., Gold, D.R., Bierzwinski, S. and Loomis, D. (1998) Mortality and ambient fine particles in Southwest Mexico City, 1993—1995. Environmental Health Perspectives, 106, 849855.CrossRefGoogle ScholarPubMed
Brunekreef, B., Hoek, G. and Spieksma, F. (2000) Relation between airborne pollen concentrations and daily cardiovascular and respiratory-disease mortality. The Lancet, 355, 15171518.CrossRefGoogle ScholarPubMed
Derbyshire, E. (1983) Origin and characteristics of some Chinese loess at two locations in China. Pp. 6990 in: Eolian Sediments and Processes (Brookfield, M.E. and Ahlbrandt, T.S., editors). Developments in Sedimentology, 38. Elsevier, Amsterdam.CrossRefGoogle Scholar
Derbyshire, E. and Mellors, T.W. (1988) Geological and geotechnical characteristics of some loess and loessic soils from China and Britain: a comparison. Engineering Geology, 25, 135175.CrossRefGoogle Scholar
Dod, R.L., Giauque, R.D. and Novakov, T. (1986) Sulphate and carbonaceous aerosols in Beijing, China. Atmospheric Environment, 20, 22712275.CrossRefGoogle Scholar
Donaldson, K., Brown, D.M., Mitchell, M.D., Beswick, P.H., Gilmore, P. and MacNee, W. (1997) Free radical activity of PM10: iron-mediated generation of hydroxyl radicals. Environmental Health Perspectives, 105, 12851289.Google ScholarPubMed
Green, D. and Barratt, B. (2001) Evaluation of TEOMtm ‘Correction Factors’ for assessing the EU Stage 1 Limit Values for PM10. Atmospheric Environment, 35, 25892593.CrossRefGoogle Scholar
Greenwell, L.L., Jones, T.P. and Richards R.J. (2002a) Collection of PM10 for toxicological investigation: comparisons between different collecting devices. Environmental Monitoring and Assessment, 79, 251273.CrossRefGoogle Scholar
Greenwell, L., Moreno, T., Jones, T.P. and Richards, R.J. (2002b)) Particle Induced Oxidative Damage is Ameliorated by Pulmonary Antioxidants. Free Radical Biology and Medicine, 32, 898905.CrossRefGoogle Scholar
Holsen, T.M., Noll, K.E., Fang, G., Lee, W. and Lin, J. (1993) Dry deposition and particle size distributions measured during the Lake Michigan Urban Air Toxics Study. Environmental Science and Technology, 27, 13271333.CrossRefGoogle Scholar
Infante, R. and Acosta, I.L. (1991) Size distribution of trace metals in Ponce, Puerto Rico air particulate matter. Atmospheric Environment , 25B, 121131.Google Scholar
Jones, T.P., BeruBe, K.A., Reynolds, L.R. and Richards, R.J. (2000) Microscopy of airborne particulates from open cast coal pits. Proceedings of Microsocopy and Microanalysis, 6, 414—145.CrossRefGoogle Scholar
Merefield, J.R., Stone, I., Barron, J. and Jones, J. (1999) Techniques for tracing fugitive mineral dusts for control of nuisance and health risk. Transactions of the Institution of Mining and Metallurgy , 108 A7781.Google Scholar
Mori, I., Nishikawa, M. and Iwasaka, Y. (1998) Chemical reaction during the coagulation of ammonium sulphate and mineral particles in the atmosphere. The Science of the Total Environment , 224, 8791.CrossRefGoogle Scholar
Pope, C.A., Dockery, D.W. and Schwartz, J. (1995) Review of epidemiological evidence of health effects of particulate air pollution. Inhalation Toxicology, 7, 118.CrossRefGoogle Scholar
Rukmangad, P.P., Phadke, K.M., Gawalpanchi, R.R. and Aggarwal, A.L. (1991) Particle size distribution and its elemental composition in the ambient air of Nagpur City. Indian Journal of Environmental Protection, 11, 409412.Google Scholar
Tsoar, H. and Pye, K. (1987) Dust transport and the question of loess formation. Sedimentology, 34, 139153.CrossRefGoogle Scholar
Xu, X., Gao, J., Dockery, D. and Chen, Y. (1994) Air pollution and daily mortality in residential areas of Beijing, China. Archives of Environmental Health, 49, 216222.CrossRefGoogle ScholarPubMed
Xu, X., Christiani, D.C. and Li, B. (1995) Association of air pollution with hospital outpatient visits in Beijing. Archives of Environmental Health, 50, 214220.CrossRefGoogle ScholarPubMed
Xuan, J. (1999) Dust emission factors for environment of Northern China. Atmospheric Environment, 33, 17671776.CrossRefGoogle Scholar