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Gamma-emitting radionuclides and metallic elements in urban dusts and sediments, Coventry, UK: implications of dosages for dispersal and disposal

Published online by Cambridge University Press:  05 July 2018

S. M. Charlesworth  and
I. D. L. Foster
S. M. Charlesworth*
Affiliation:
Centre for Environmental Research and Consultancy, Geography and Environmental Science, Coventry University, Priory Street, Coventry CV1 5FB, UK
I. D. L. Foster
Affiliation:
Geography Department, Rhodes University, Grahamstown 6140, South Africa
*
*E-mail: [email protected]
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Abstract

Gully pot sediments and pavement and road gutter dusts have been collected from the city of Coventry in the West Midlands, UK. These samples have been subjected to metallic element analysis and the activity of a number of gamma-emitting radionuclides have been measured in order to assess whether they exceed published trigger or action levels, and whether their disposal or dispersal may have implications for receiving landfills and/or water courses. Results indicate above-background levels of metallic elements in dusts and sediments with Cu and Zn exceeding ICRCL action levels in some cases. The highest activities of some radionuclides are found in road gutter and street dusts and the lowest activities are found in gully pot sediments. Road dusts are more likely to be recirculated into the ambient air by passing traffic and could potentially pose a risk to pedestrians. The effective dose rates calculated for these dusts and sediments indicate that some samples approach and even exceed the 1 mSv y—1 limit to members of the public recommended by ICRP (1991). Some individual nuclides exceed their clearance levels laid down in the revised basic safety standards of the 1993b Radioactive Substances Act, 1993 (DoETR, 1999), by as much as 2.5 times. This is especially true of 210Pbun and 7Be, two fallout nuclides, and also of 40K.

Keywords

radionuclidesCoventryUKgamma-emitting
Type
Research Article
Information
Mineralogical Magazine , Volume 69 , Issue 5 , October 2005 , pp. 759 - 767
Copyright
Copyright © The Mineralogical Society of Great Britain and Ireland 2005

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References

Appleby, P.G., Nolan, P.J., Gifford, D.W., Godfrey, M.J., Oldfield, F., Anderson, N.J. and Battarbee, R.W. (1986) 210Pb dating by low background gamma counting. Hydrobiologia, 141, 21—27.CrossRefGoogle Scholar
Charlesworth, S.M. and Lees, J.A. (1999) The distribution of heavy metals in deposited dusts and sediments, Coventry, UK. Environmental Geochemistry and Health, 21, 97 – 115.Google Scholar
Charlesworth, S.M., Everett, M., Mc Carthy, R., Ordonez, A. and de Miguel, E. (2003) A comparative study of heavy metal concentration and distribution in deposited street dusts in a large and a small urban area: Birmingham and Coventry, West Midlands, UK. Environment International, 29, 563–57.CrossRefGoogle Scholar
Colmenero, S.L., Montero Cabrera, M.E., Villalba, L., Renteria Villalobos, M., Torres Moye, E., Garcia Leon, M., Garcia-Tenario, R., Mireles Garcia, F., Herrera Peraza, E.F. and Sanchez Aroche, D. (2004) Uranium-238 and thorium-232 series concentrations in soil, radon-222 indoor and drinking water concentrations and dose assessment in the city of Aldama, Chihuahua, Mexico. Journal of Environmental Radioactivity, 11, 205–219.CrossRefGoogle Scholar
Dalgleish, H. (1994) Caesium-137 distribution and uptake in an agricultural environment. Unpublished PhD Thesis, Coventry University, UK.Google Scholar
DEFRA (Department of Environment, Food and Rural Affairs) and EA (Environment Agency) (2002) Assessment of risks to human health from land contamination: An overview of the development of guideline values and related research. Report CLR7, UK.Google Scholar
DoETR (Department of the Environment, Transport and the Regions) (1999) The Radioactive Substances Act, 1993: Implementing the revised basic safety standards Directive Euratom 96/29. Defra Publication, UK.Google Scholar
Ferreira-Baptista, L. and De Miguel, E. (2005) Geochemistry and risk assessment of street dust in Luanda, Angola, a tropical urban environment. Atmospheric Environment, 39, 4501–4512.CrossRefGoogle Scholar
Foster, I.D.L. (1995) Lake and reservoir bottom-sediments as a source of soil erosion and sediment transport data in the UK. Pp. 265–283 in: Sediment and Water Quality in River Catchments (Foster, I.D.L., Gurnell, A.M. and Webb, B.W., editors). Wiley, Chichester, UK.Google Scholar
Foster, I.D.L., Dalgleish, H., Dearing, J.A. and Jones, E.D. (1994) Quantifying soil erosion and sediment transport in drainage basins; some observations on the use of 137Cs. IAHS Publications, 224, 55–6.Google Scholar
Foster, I.D.L., Lees, J.A., Jones, A.R., Chapman, A.S., Turner, S.E. and Hodgkinson, R.A. (2002) The possible role of agricultural land drains in sediment delivery to a small reservoir, Worcestershire UK; a multiparameter tracing study. Pp. 433–442 in: The Structure, Function and Management Implications of Fluvial Sedimentary Systems (Dyer, F.J., Thorns, M.C. and Olley, J.M., editors). IAHS, volume 276, International Association of Hydrological Sciences, France.Google Scholar
ICRCL (Inter-Departmental Committee on the redevelopment of Contaminated Land) (1983) Guidance on the assessment and redevelopment of contaminated land. ICRCL Paper 59/83, Department of the Environment, London.Google Scholar
ICRP (1991) 1990 Recommendations of the International Commission on Radiological Protection; ICRP publication 60. Annals of ICRP, 21, 1–3.Google Scholar
Macklin, M.G. (1992) Metal pollution of soils and sediments: a geographic perspective. Pp 172–195 in: Managing the Human Impacts on the Natural Environment: Patterns and Processes (Newson, M., editor). Belhaven Press, London.Google Scholar
Merefield, J.R., Stone, I.M., Roberts, J., Jones, J., Barr, J. and Dean, A. (2000) Fingerprinting airborne particles for identifying provenance. Pp. 85–100 in: Tracers in Geomorphology (Foster, I.D.L., editor). Wiley, Chichester, UK.Google Scholar
Murray, A.S., Marten, R., Johnston, A. and Martin, P. (1987) Analysis for naturally occurring radionuclides at environmental concentrations by gamma spectrometry. Journal of Radioanalytical and Nuclear Chemistry, 115, 263–288.CrossRefGoogle Scholar
QUARG (Quality of Urban Air Review Group) (1996) Airborne paniculate matter in the United Kingdom. Department of the Environment, UK.Google Scholar
Robertson, D.J., Taylor, K.G. and Hoon, S.R. (2003) Geochemical and mineral magnetic characterisation of urban sediment particulates, Manchester, UK. Applied Geochemistry, 18, 269–282.CrossRefGoogle Scholar
Salomons, W. and Forstner, U. (1984) Metals in the hydrocycle. Springer-Verlag.CrossRefGoogle Scholar
Sutherland, R.A. and Tolosa, C.A. (2000) Multi-element analysis of road-deposited sediment in an urban drainage basin, Honolulu, Hawaii. Environmental Pollution, 110, 483–495.CrossRefGoogle Scholar
UN Population Division (2005) Population Challenges and Development Goals, http://www.un.org/esa/population/publications/popchallenges/Population_Challenges.pdfGoogle Scholar
UNSCEAR (2000) Sources and effects of ionising radiation Annex A: Dose Assessment Methodologies. United Nations Scientific Committee on the Effects of Atomic Radiation. UNSCEAR 2000, New York, USA.Google Scholar
Vaze, J. and Chiew, F.H.S. (2002) Experimental study of pollutant accumulation on an urban road surface. Urban Water, 4, 379–389.CrossRefGoogle Scholar