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Structure property relationship in (TiZrNbCu)1−xNix metallic glasses

Published online by Cambridge University Press:  26 June 2018

Emil Babić ,
Damir Pajić ,
Krešo Zadro ,
Katica Biljaković ,
Vesna Mikšić Trontl ,
Petar Pervan ,
Damir Starešinić ,
Ignacio A. Figueroa ,
Ahmed Kuršumović  and
Štefan Michalik
...Show all authors
Emil Babić
Affiliation:
Department of Physics, Faculty of Science, Zagreb HR-10002, Croatia
Damir Pajić
Affiliation:
Department of Physics, Faculty of Science, Zagreb HR-10002, Croatia
Krešo Zadro
Affiliation:
Department of Physics, Faculty of Science, Zagreb HR-10002, Croatia
Katica Biljaković
Affiliation:
Institute of Physics, Zagreb HR-10001, Croatia
Vesna Mikšić Trontl
Affiliation:
Institute of Physics, Zagreb HR-10001, Croatia
Petar Pervan
Affiliation:
Institute of Physics, Zagreb HR-10001, Croatia
Damir Starešinić
Affiliation:
Institute of Physics, Zagreb HR-10001, Croatia
Ignacio A. Figueroa
Affiliation:
Institute for Materials Research-UNAM, Ciudad Universitaria Coyoacan, Ciudad de Mexico C.P. 04510 D.F., Mexico
Ahmed Kuršumović
Affiliation:
Department of Materials Science & Metallurgy, University of Cambridge, Cambridge CB3 0FS, U.K.
Štefan Michalik
Affiliation:
Diamond Light Source Ltd., Harwell Science and Innovation Campus, DidcotOX11 0DE, U.K.
Andrea Lachová
Affiliation:
Institute of Physics, Faculty of Science, P.J. Šafárik University in Košice, Košice 041 54, Slovak Republic
György Remenyi
Affiliation:
Institut Neel, Universite Grenoble Alpes, Grenoble F-38042, France
Ramir Ristić*
Affiliation:
Department of Physics, University of Osijek, Osijek HR-3100, Croatia
*
a)Address all correspondence to this author. e-mail: [email protected]
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Abstract

The atomic structure, electronic structure, and physical properties of (TiZrNbCu)1−xNix (x ≤ 0.5) metallic glasses (MGs) were studied in both the high-entropy (0 < x < 0.35) and the higher Ni concentration range (x ≥ 0.35). Atomic structure studies performed with X-ray diffraction and synchrotron powder diffraction provided average atomic volumes, structure factors, radial distribution functions, coordination numbers, and packing densities. Electronic structure studies performed using photoemission spectroscopy and low-temperature specific heat provided information about the electronic density of states within the valence band and at the Fermi level and also about interatomic bonding and atomic vibrations [from the Debye temperature and the boson peak (BP)]. Variations of both atomic structure and electronic structure with x showed a clear change for x ≥ 0.35, which corresponds to a valence electron number ≥7.4. All physical properties, namely, thermal stability parameters, Debye temperatures, BPs, magnetic, elastic, and electronic transport properties, change their concentration-dependence for x ≥ 0.35. The results are compared with those for binary and ternary MGs of the same elements.

Keywords

amorphouselectronic structureinteratomic arrangements
Type
Invited Review
Information
Journal of Materials Research , Volume 33 , Issue 19: Focus Issue: Fundamental Understanding and Applications of High-Entropy Alloys , 14 October 2018 , pp. 3170 - 3183
Copyright
Copyright © Materials Research Society 2018 

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Footnotes

This section of Journal of Materials Research is reserved for papers that are reviews of literature in a given area.

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