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Miscible displacements in capillary tubes. Part 1. Experiments

Published online by Cambridge University Press:  26 April 2006

P. Petitjeans
Affiliation:
Department of Aerospace Engineering, University of Southern California, Los Angeles, CA 90090-1191, USA
T. Maxworthy
Affiliation:
Laboratoire de Physique et Mecanique des Milieux Heterogenes, Ecole Superieure de Physique et Chimie Industrielles, 10, Rue Vauquelin, F-75231, Paris cedex 05, France

Abstract

Experiments have been performed, in capillary tubes, on the displacement of a viscous fluid (glycerine) by a less viscous one (a glycerine–water mixture) with which it is miscible in all proportions. A diagnostic measure of the amount of viscous fluid left behind on the tube wall has been found, for both vertical and horizontal tubes, as a function of the Péclet (Pe) and Atwood (At) numbers, as well as a parameter that is a measure of the relative importance of viscous and gravitational effects. The asymptotic value of this diagnostic quantity, for large Pe and an At of unity, has been found to agree with that found in immiscible displacements, while the agreement with the numerical results of Part 2 (Chen & Meiburg 1966), over the whole range of At, is very good. At values of the average Pe greater than 1000 a sharp interface existed so that it was possible to make direct comparisons between the present results and a prior experiment with immiscible fluids, in particular an effective surface tension at the diffusing interface could be evaluated. The effect of gravity on the amount of viscous fluid left on the tube wall has been investigated also, and compared with the results of Part 2. A subsidiary experiment has been performed to measure both the average value of the diffusion coefficient between pure glycerine and several glycerine–water mixtures, in order to be able to calculate a representative Péclet number for each experiment, and the local value as a function of the local concentration of glycerine, in the dilute limit.

Type
Research Article
Copyright
© 1996 Cambridge University Press

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References

Bensimon, D., Kadanoff, L. P., Liang, S., Shraiman, B. I. & Tang, C. 1986 Viscous flows in two dimensions. Rev. Mod. Phys. 58, 977.Google Scholar
Brady, J. F. & Koch, D. L. 1988 Dispersion in porous media. In Disorder and Mixings (ed. E. Guyon et al.). NATO ASI Series E, Academic.
Chen, C.-H. & Meiburg, E. 1996 Miscible displacements in a capillary tube. Part 2. Numerical simulations. J. Fluid Mech. 326, 57 (referred to herein as Part 2).Google Scholar
Chouke, R. L., Meurs, P. van & Pol, C. van der 1959 The instability of slow, immiscible, viscous liquid-liquid displacements in permeable media. Trans. AIME 216, 188.Google Scholar
Clift, R., Grace, J. R. & Weber, M. E. 1978 Bubbles, Drops and Particles. Academic.
Cox, B. G. 1962 On driving a viscous fluid out of a tube. J. Fluid Mech. 14, 81.Google Scholar
Davis, H. T. 1988 A theory of tension at a miscible displacement front. In Numerical Simulation in Oil Recovery (ed. M. Wheeler). Springer.
Goldsmith, H. L. & Mason, S. G. 1963 The flow of suspensions through tubes, Part II. Single large bubbles. J. Colloid Sci. 18, 237.Google Scholar
Homsy, G. M. 1987 Viscous fingering in porous media. Ann. Rev. Fluid Mech. 19, 271.Google Scholar
Hu, H. H. & Joseph, D. D. 1991 Interfacial tension between miscible liquids. Preprint of the Dept, of Aero. Engng., University of Minnesota.
Joseph, D. D. 1990 Fluid dynamics of two miscible liquids with diffusion and gradient stress. Eur. J. Mech. B/Fluids 9, 565.Google Scholar
Korteweg, D. J. 1901 Sur la forme que prennant les equation du movement des fluides si l'on tient compte des forces capillaires causees par des variations de densite. Arch. Neerl. Sci. Ex. Nat. (ii) 6, 1.Google Scholar
Kurowski, P. & Misbah, C. 1994 A non-standard effect of diffusion on a fictitious front between miscible fluids. Eur. Phys. Letts. 29, 309.Google Scholar
Maxworthy, T. 1989 Experimental study of instability in a Hele-Shaw cell. Phys. Rev. A 39, 3863.Google Scholar
Meiburg, E. & Homsy, G. M. 1988 Nonlinear, unstable, viscous fingers in Hele-Shaw flows. Part 2: Numerical simulations Phys. Fluids 31, 429.Google Scholar
Petitjeans, P. 1996 Une tension de surface pour les fluides miscibles. C. R. Acad. Sci. Paris serie IIb 322, 673.Google Scholar
Reinelt, D. A. & Saffman, P. G. 1985 The penetration of a finger into a viscous fluid in a channel and tube. SIAM J. Sci. Statist. Comput. 6, 582.Google Scholar
Saffman, P. G. 1986 Viscous fingering in Hele-Shaw cells. J. Fluid Mech. 173, 73.Google Scholar
Saffman, P. G. & Taylor, G. I. 1958 The penetration of a finger into a porous medium in a Hele-Shaw cell containing a more viscous liquid. Proc. Roy. Soc. Lond. A 245, 312.Google Scholar
Tan, C. T. & Homsy, G. M. 1986 Stability of miscible displacements in porous media: rectilinear flow. Phys. Fluids 29, 3549.Google Scholar
Taylor, G. I. 1961 Deposition of a viscous fluid on the wall of a tube. J. Fluid Mech. 10, 161.Google Scholar
Templeton, C. C. 1953 A study of displacements in microscopic capillaries. Petrol. Trans. AIME 33, 162.Google Scholar
Yortsos, Y. C. & Zeybek, M. 1988 Dispersion driven instability in miscible displacement in porous media. Phys. Fluids 31, 3511.Google Scholar
Zimmerman, W. & Homsy, G. M. 1991 Nonlinear viscous fingering in miscible displacement with anisotropic dispersion. Phys. Fluids A 3, 1859.Google Scholar