Hostname: page-component-586b7cd67f-2plfb Total loading time: 0 Render date: 2024-11-28T05:07:11.535Z Has data issue: false hasContentIssue false

Diffusive and phase change instabilities in a ternary mushy layer

Published online by Cambridge University Press:  12 November 2014

Peter Guba
Affiliation:
Department of Applied Mathematics and Statistics, Faculty of Mathematics, Physics and Informatics, Comenius University, 842 48 Bratislava 4, Slovakia
Daniel M. Anderson*
Affiliation:
Department of Mathematical Sciences, George Mason University, Fairfax, VA 22030, USA Applied and Computational Mathematics Division, National Institute of Standards and Technology, Gaithersburg, MD 20899-8910, USA
*
Email address for correspondence: [email protected]

Abstract

We analyse the stability of a mushy layer during the directional solidification of a ternary alloy. Our model includes diffusive and convective transport of heat and solutes, coupled by an equilibrium thermodynamic constraint of the ternary phase diagram. The model contains phase change effects due to latent-heat release, solute rejection and background solidification. We identify novel convective instabilities, both direct and oscillatory, which are present under statically stable conditions. We examine these instabilities asymptotically by simplifying to a thin mushy layer with small growth rates. We also discuss numerical results for the full problem, confirming the asymptotic predictions and providing the stability characteristics outside the small-growth-rate approximation. A physical explanation for these instabilities in terms of parcel arguments is proposed, indicating that the instability mechanisms generally involve different rates of solute diffusion, different rates of solute rejection and different background solute distributions induced by the initial alloy composition.

Type
Papers
Copyright
© 2014 Cambridge University Press 

Access options

Get access to the full version of this content by using one of the access options below. (Log in options will check for institutional or personal access. Content may require purchase if you do not have access.)

References

Aitta, A., Huppert, H. & Worster, M. G. 2001 Diffusion-controlled solidification of a ternary melt from a cooled boundary. J. Fluid Mech. 432, 201217.CrossRefGoogle Scholar
Amberg, G. & Homsy, G. M. 1993 Nonlinear analysis of buoyant convection in binary solidification with application to channel formation. J. Fluid Mech. 252, 7998.Google Scholar
Anderson, D. M. 2003 A model for diffusion-controlled solidification of ternary alloys in mushy layers. J. Fluid Mech. 483, 165197.CrossRefGoogle Scholar
Anderson, D. M., McFadden, G. B., Coriell, S. R. & Murray, B. T. 2010 Convective instabilities during the solidification of an ideal ternary alloy in a mushy layer. J. Fluid Mech. 647, 309333.Google Scholar
Anderson, D. M. & Schulze, T. P. 2005 Linear and nonlinear convection in solidifying ternary alloys. J. Fluid Mech. 545, 213243.Google Scholar
Anderson, D. M. & Worster, M. G. 1995 Weakly nonlinear analysis of convection in mushy layers during the solidification of binary alloys. J. Fluid Mech. 302, 307331.Google Scholar
Anderson, D. M. & Worster, M. G. 1996 A new oscillatory instability in a mushy layer during the solidification of binary alloys. J. Fluid Mech. 307, 245267.Google Scholar
Beckermann, C. & Viskanta, R. 1993 Mathematical modeling of transport phenomena during alloy solidification. Appl. Mech. Rev. 46, 127.Google Scholar
Bennon, W. D. & Incropera, F. P. 1987 A continuum model for momentum, heat and species transport in binary solid–liquid phase change systems-I. Model formulation. Intl J. Heat Mass Transfer 30, 21612170.Google Scholar
Bloomfield, L. J. & Huppert, H. E. 2003 Solidification and convection of a ternary solution cooled from the side. J. Fluid Mech. 489, 269299.Google Scholar
Boyd, J. P. 2001 Chebyshev and Fourier Spectral Methods. Dover.Google Scholar
Fujii, T., Poirier, D. R. & Flemings, M. C. 1979 Macrosegregation in a multicomponent low alloy steel. Metall. Trans. B 10, 331339.Google Scholar
Hughes, D. W. 1985 Magnetic buoyancy instabilities for a static plane layer. Geophys. Astrophys. Fluid Dyn. 32, 273316.Google Scholar
Krane, M. J. M. & Incropera, F. P. 1997 Solidification of ternary metal alloys-II. Predictions of convective phenomena and solidification behavior in Pb–Sb–Sn alloys. Intl J. Heat Mass Transfer 40, 38373847.CrossRefGoogle Scholar
Krane, M. J. M., Incropera, F. P. & Gaskell, D. R. 1997 Solidification of ternary metal alloys-I. Model development. Intl J. Heat Mass Transfer 40, 38273835.Google Scholar
Krane, M. J. M., Incropera, F. P. & Gaskell, D. R. 1998 Solidification of a ternary metal alloy: a comparison of experimental measurements and model predictions in a Pb–Sb–Sn system. Metall. Mater. Trans. A 29, 843853.Google Scholar
Mehrabian, R. & Flemings, M. C. 1970 Macrosegregation in ternary alloys. Metall. Mater. Trans. B 1, 455464.Google Scholar
Mehrabian, R., Keane, M. & Flemings, M. C. 1970 Interdendritic fluid flow and macrosegregation; influence of gravity. Metall. Trans. 1, 12091220.Google Scholar
Nield, D. A. 1968 Onset of thermohaline convection in a porous medium. Water Resour. Res. 3, 553560.Google Scholar
Roberts, P. H. & Loper, D. E. 1979 On the diffusive instability of some simple steady magnetohydrodynamic flows. J. Fluid Mech. 90, 641668.Google Scholar
Schneider, M. C. & Beckermann, C. 1995 Formation of macrosegregation by multicomponent thermosolutal convection during the solidification of steel. Metall. Mater. Trans. A 26, 23732388.Google Scholar
Sivashinsky, G. 1983 Negative viscosity effect in large-scale turbulence. Long-wave instability of a periodic system of eddies. Phys. Lett. A 95, 152154.Google Scholar
Sivashinsky, G. & Yakhot, V. 1985 Negative viscosity effect in large-scale flows. Phys. Fluids 28, 10401042.CrossRefGoogle Scholar
Starr, V. P. 1968 Physics of Negative Viscosity Phenomena. McGraw-Hill.Google Scholar
Thompson, A. F., Huppert, H. E., Worster, M. G. & Aitta, A. 2003 Solidification and compositional convection of a ternary alloy. J. Fluid Mech. 497, 167199.Google Scholar
West, D. R. F. 1982 Ternary Equilibrium Diagrams, 2nd edn. Chapman and Hall.Google Scholar