We show that linearly repetitive weighted Delone sets in groups of polynomial growth have a uniquely ergodic hull. This result applies in particular to the linearly repetitive weighted Delone sets in homogeneous Lie groups constructed in the companion paper [S. Beckus, T. Hartnick and F. Pogorzelski. Symbolic substitution beyond Abelian groups. Preprint, 2021, arXiv:2109.15210] using symbolic substitution methods. More generally, using the quasi-tiling method of Ornstein and Weiss, we establish unique ergodicity of hulls of weighted Delone sets in amenable unimodular locally compact second countable groups under a new repetitivity condition which we call tempered repetitivity. For this purpose, we establish a general sub-additive convergence theorem, which also has applications concerning the existence of Banach densities and uniform approximation of the spectral distribution function of finite hopping range operators on Cayley graphs.