We present a characterization of the performance of an ultrashort laser pulse driven DC photoelectron gun based on the thermionic emission gun design of Togawa et al. [Togawa, K., Shintake, T., Inagaki, T., Onoe, K. & Tanaka, T. (2007). Phys Rev Spec Top-AC10, 020703]. The gun design intrinsically provides adequate optical access and accommodates the generation of ∼1 mm2 electron beams while contributing negligible divergent effects at the anode aperture. Both single-photon (with up to 20,000 electrons/pulse) and two-photon photoemission are observed from Ta and Cu(100) photocathodes driven by the harmonics (∼4 ps pulses at 261 nm and ∼200 fs pulses at 532 nm, respectively) of a high-power femtosecond Yb:KGW laser. The results, including the dependence of the photoemission efficiency on the polarization state of the drive laser radiation, are consistent with expectations. The implications of these observations and other physical limitations for the development of a dynamic transmission electron microscope with sub-1 nm·ps space-time resolution are discussed.

Radio-frequency (RF) photoinjector-based relativistic ultrafast electron diffraction (UED) is a promising new technique that has the potential to probe structural changes at the atomic scale with sub-100 fs temporal resolution in a single shot. We analyze the limitations on the temporal and spatial resolution of this technique considering the operating parameters of a standard 1.6 cell RF gun (which is the RF photoinjector used for the first experimental tests of relativistic UED at Stanford Linear Accelerator Center; University of California, Los Angeles; Brookhaven National Laboratory), and study the possibility of employing novel RF structures to circumvent some of these limits.

This paper reports on a novel approach for producing high energy femtosecond pulses without external amplification. The so-called chirped-pulse oscillator (CPO) concept is based on an extended-cavity oscillator, operating at small net positive intracavity group delay dispersion (GDD), over a broad spectral range by the use of chirped multilayer mirrors. The resultant chirped picosecond pulses are compressed by a dispersive delay line external to the laser cavity. Utilizing this technique, sub-30 fs pulses with an energy exceeding 200 nJ at a repetition rate of 11 MHz were produced. The demonstrated peak power in excess of 5 MW is the highest ever achieved from a cw-pumped laser and is expected to be scaleable to tens of megawatts by increasing the pump power and/or decreasing the repetition rate. The demonstrated source allows micromachining of any materials under relaxed focusing conditions.

Using the technique of tight-binding electron–ion dynamics, we have calculated the response of crystalline GaAs when a femtosecond laser pulse excites 1–20% of the valence electrons. Above a threshold fluence, which corresponds to promotion of about 12% of the valence electrons to the conduction band, the lattice is destabilized and the band gap collapses to zero. This result supports the conclusion that structural changes on a subpicosecond time scale observed in pump-probe experiments are of a nonthermal nature.