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Performance evaluation of neutron detectors incorporating intrinsic Gd using a GEANT4 modeling approach

Published online by Cambridge University Press:  28 October 2011

Abigail A. Bickley
Affiliation:
Department of Engineering Physics, Air Force Institute of Technology, 2950 Hobson Way, Wright-Patterson Air Force Base, OH 45433-7765, U.S.A.
Christopher Young
Affiliation:
Department of Engineering Physics, Air Force Institute of Technology, 2950 Hobson Way, Wright-Patterson Air Force Base, OH 45433-7765, U.S.A.
Benjamin Thomas
Affiliation:
Department of Engineering Physics, Air Force Institute of Technology, 2950 Hobson Way, Wright-Patterson Air Force Base, OH 45433-7765, U.S.A.
John W. McClory
Affiliation:
Department of Engineering Physics, Air Force Institute of Technology, 2950 Hobson Way, Wright-Patterson Air Force Base, OH 45433-7765, U.S.A.
Peter A. Dowben
Affiliation:
Department of Physics and Astronomy, University of Nebraska - Lincoln, 855 North 16th St, Lincoln, NE 68588-0299, U.S.A.
James C. Petrosky
Affiliation:
Department of Engineering Physics, Air Force Institute of Technology, 2950 Hobson Way, Wright-Patterson Air Force Base, OH 45433-7765, U.S.A.
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Abstract

Solid-state neutron detectors from heterostructures that incorporate Gd intrinsically or as a dopant may significantly benefit from the high thermal neutron capture cross section of gadolinium. Semiconducting devices with Gd atoms can act as a neutron capture medium and simultaneously detect the electronic signal that characterizes the interaction. Neutron capture in natural isotopic abundance gadolinium predominantly occurs via the formation of 158mGd, which decays to the ground state through the emission of high-energy gamma rays and an internal conversion electron. Detection of the internal conversion electron and/or the subsequent Auger electron emission provides a distinct and identifiable signature that neutron capture has occurred. Ensuring that the medium responds to these emissions is imperative to maximizing the efficiency and separating out other interactions from the radiation environment. A GEANT4 model, which includes incorporation of the nuclear structure of Gd, has been constructed to simulate the expected device behavior. This model allows the energy deposited from the decay of the meta-stable state to be localized and transported, providing for analysis of various device parameters. Device fabrication has been completed for Gd doped HfO2 on n-type silicon, Gd2O3 on p-type silicon and Gd2O3 on SiC for validation of the code. A preliminary evaluation of neutron detection capabilities of these devices using a GEANT4 modeling approach is presented.

Type
Research Article
Copyright
Copyright © Materials Research Society 2011

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References

REFERENCES

1. Kramer, D., “DOE begins rationing helium-3”, Physics Today, 2225, June 2010.Google Scholar
2. Chadwick, M.B., Oblozinsky, P., Herman, M. et al. ., “ENDF/B-VII.0: Next Generation Evaluated Nuclear Data Library for Nuclear Science and Technology”, Nuclear Data Sheets, vol. 107, pp. 29313060, 2006.Google Scholar
3. Ge, Z.G., Zhuang, Y.X., Liu, T.J., Zhang, J.S., Wu, H.C., Zhao, Z.X., Xia, H.H., “The Updated Version of Chinese Evaluated Nuclear Data Library (CENDL-3.1)”, Proc. International Conference on Nuclear Data for Science and Technology, Jeju Island, Korea, April 26-30, 2010 (in press).Google Scholar
4. Ketsman, I., Losovyj, Y.B., Sokolov, A., Tang, J., Wang, Z., Natta, M.L., Brand, J.I., Dowben, P.A., Appl. Surf. Sci. 254, 4308 (2008).Google Scholar
5. Losovyj, Y.B., Wooten, D., Santana, J.C., An, J.M., , Belashchenko, K.D., Lozova, N., Petrosky, J., Sokolov, A., Tang, J., Wang, W., Arulsamy, N., Dowben, P.A., J. Phys. Condens. Matter 21, 045602 (2009).Google Scholar
6. Schultz, D., Blasy, B., Santana, J.C., Young, C., Petrosky, J.C., McClory, J.W., LaGraffe, D., Brand, J.I., Tang, J., Wang, W., Schemm, N., Balkir, S., Bauer, M., Ketsman, I., Fairchild, R.W., Losovyj, Y.B., Dowben, P.A., J. Phys. D: Appl. Phys. 43, 075502 (2010).Google Scholar
7. Monte-Carlo Simulation of Electron Trajectory in Solids (CASINO), accessed August 2009. Available: http://www.gel.usherbrooke.ca/casino/index.html.Google Scholar
8. Thomas, B., “Neutron Detection Using Gadolinium-Based Diodes,” MS thesis, Department of Engineering Physics, Air Force Institute of Technology, Wright-Patterson AFB, OH, 2011.Google Scholar
9. Young, C., “Gadolinium Oxide / Silicon Thin Film Heterojunction Solid-State Neutron Detector,” MS thesis, Department of Engineering Physics, Air Force Institute of Technology, Wright-Patterson AFB, OH, 2010.Google Scholar
10. Agostinelli, S., et al. ., Nucl. Instrum. Methods Phys. Res. A 506, 250 (2003).Google Scholar
11. Helmer, R.G., Nuclear Data Sheets 101, 325 (2004).Google Scholar
12. GEANT4 Collaboration, “Data files for photon evaporation - version 2.1”, released February 2011. Available: http://geant4.web.cern.ch/geant4/support/download.shtml Google Scholar
13. Ali, M.A., Khitrov, V.A., Kholnov, Y.V., Sukhovoj, A.M., Vojnov, A.V., J. Phys. G Nucl. Part. Phys. 20, 1943 (1994).Google Scholar
14. Islam, M.A., Kennett, T.J., Prestwich, W.V., Phys. Rev. C 25, 3184 (1982).Google Scholar
15. Firestone, R.B., Choi, H.D., Lindstrom, R.M., Molnar, G.L., Mughabghab, S.F., Paviotti-Corcuera, R., et al. ., Database of prompt gamma rays from slow neutron capture for elemental analysis, (Lawrence Berkeley National Laboratory, California, 2004) p. 132.Google Scholar
16. GEANT4 Collaboration, “Physics Reference Manual geant4.9.4”, released December 2010, p 499. Available: http://geant4.web.cern.ch/geant4/UserDocumentation/UsersGuides/PhysicsReferenceManual/fo/PhysicsReferenceManual.pdf Google Scholar
17. Rosel, F., Fries, H.M., Alder, K. and Pauli, H.C., At. Data Nucl. Data Tables 21 (1978).Google Scholar
18. Kinsey, et al. ., Can. J. Phys. 31, 1051 (1953).Google Scholar
19. Groshev, et al. ., Atomnaya Energiya 4, No 1, 5 (1958).Google Scholar
20. Becvar, F., Krticka, M., Tomandl, I., Honzatko, J., Voss, F., Wisshak, K., Kappeler, F., AIP Conf. Proc. 529, 657 (2000).Google Scholar